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ACS applied materials & interfaces v.9 no.2, 2017년, pp.1183 - 1188   SCI SCIE
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Solvent Accommodation: Functionalities Can Be Tailored Through Co-Crystallization Based on 1:1 Coronene-F4TCNQ Charge-Transfer Complex

Zhang, Jing (Key Laboratory for Organic Electronics and Information Displays & Institute of Advanced Materials, Jiangsu National Synergetic Innovation Center for Advanced Materials, Nanjing University of Posts & Telecommunications, 9 Wenyuan Road, Nanjing 210023, ); Liu, Guangfeng ( School of Materials Science and Engineering, Nanyang Technological University, Singapore 639798, ); Zhou, Yecheng ( School of Chemistry, The University of Melbourne, Parkville, Victoria 3010, ); Long, Guankui ( School of Materials Science and Engineering, Nanyang Technological University, Singapore 639798, ); Gu, Peiyang ( School of Materials Science and Engineering, Nanyang Technological University, Singapore 639798, ); Zhang, Qichun ( School of Materials Science and Engineering, Nanyang Technological University, Singapore 639798, );
  • 초록  

    Because organic donor/acceptor blending systems play critical roles in ambipolar transistors, photovoltaics, and light-emitting transistors, it is highly desirable to precisely tailor the stacking of cocrystals toward different intrinsic structures and physical properties. Here, we demonstrated that the structure-stacking modes and electron-transport behaviors of coronene-F4TCNQ cocrystals (1:1) can be tuned through the solvent accommodation. Our results clearly show that the solvent accommodation not only enlarges the inner mixed packing (...DAD···) distances, leading to the depressed short-contact interactions including the side-by-side and face-by-face intermolecular interactions, but also switches off electron-transport behavior of coronene-F 4 TCNQ cocrystals (1:1) in ambient atmosphere. Graphic Abstract ACS Electronic Supporting Info


  • 주제어

    solvent accommodation .   co-crystallization .   supramolecular system .   depressed short contact .   electron transport.  

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