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Inorganic chemistry communications v.85, 2017년, pp.105 - 109   SCI SCIE
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Two transition metal coordination polymers constructed from 1,4-naphthalenedicarboxylate and N/O-donor auxiliary ligands: Syntheses, structures and magnetic property

Zou, Guo-Dong (College of Chemistry and Chemical Engineering, Xinyang Normal University, Xinyang, Henan 464000, PR China ) ; Tian, Chong-Bin (State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, The Chinese Academy of Sciences, Fuzhou, Fujian 350002, PR China ) ; Yu, Xiao-Chen (College of Chemistry and Chemical Engineering, Xinyang Normal University, Xinyang, Henan 464000, PR China ) ; Lu, Jing (College of Chemistry and Chemical Engineering, Xinyang Normal University, Xinyang, Henan 464000, PR China ) ; Chen, Ming (College of Chemistry and Chemical Engineering, Xinyang Normal University, Xinyang, Henan 464000, PR China ) ;
  • 초록  

    Abstract Two transition metal coordination polymers (CPs), namely, Cd(1,4-NDC)(py) ( 1 ), Co 2 (1,4-NDC) 2 (DMF) 2 ( 2 ) (1,4-NDCH 2 = 1,4-naphthalenedicarboxylic acid, py=pyridine, DMF= N , N -dimethylformamide) have been synthesized and characterized. Compound 1 contains one-dimensional chains, which are further linked by the NDC 2− ligands to form a three-dimensional framework with a 5,5T2 topology network. There exist two types of left-hand helical chains interconnected to each other through the Cd(II) center in compound 1 . Although compound 2 has been reported previously, in this work the synthetic method of 2 is modified to obtain high quality crystals. In addition, the magnetic property of compound 2 is investigated, which shows the metamagnetic behavior induced by the external field. Highlights There exist two types of left-hand helical chains in compound 1 . Compound 1 possesses 5,5T2 topology network. Compound 2 shows the metamagnetic behavior induced by the external field. Graphical abstract Two transition-metal coordination polymers (CPs) have been synthesized and characterized. The metamagnetic behavior of the Co-based CP is investigated. [DISPLAY OMISSION]


  • 주제어

    Coordination polymer .   Crystal structure .   Metamagnetism .   Transition metal ion.  

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